In 2012, Pope parted ways with Hey Monday to pursue a solo career, and around the same time auditioned for and was accepted on NBC's reality singing competition The Voice. Choosing to join judge Blake Shelton's team, Pope eventually won, beating out teammate Terry McDermott. Pope signed to Universal Music Group and worked on her debut solo album, Frame by Frame, which was released in October 2013. She toured extensively behind the release, spending much of 2014 on the road opening shows for Tim McGraw and Dierks Bentley. The following year, Pope returned with the single "I Am Invincible." Another single, "Think of You," a duet with Chris Young, followed in January 2016. It became a radio favorite and went all the way to number one on the country airplay survey and then went gold. That June, Pope released a four-song EP, fittingly titled Summer.
She then parted ways with her label and signed with Fusion Music. In 2018, she marked the change with the single "Take You Home." Also that year, she returned to The Voice, working as an advisor to coach Kelly Clarkson's team. A second full-length album, the Corey Crowder-produced Stages, arrived in February 2019, and included "Take You Home" as well as the single "If My Heart Had a Heart." It reached number 39 on the Billboard Top Country Albums chart. She returned in June 2020 with the all-acoustic album Rise and Shine. ~ Matt Collar, Rovi